Three-dimensional rolling is a novel forming process for three-dimensional surface parts, which combines the rolling process with multi-point forming technology. This process employs a pair of forming rolls as a forming tool; the residual stress of sheet metal makes the sheet metal generate three-dimensional deformation by controlling the nonuniform distribution of roll gap of the forming rolls. In this article, two types of forming processes are investigated for three-dimensional surface parts with the same target shape in different roll adjusting radius. The roll adjusting radius of a forming process is much larger than the target transverse curvature radius of the forming part, and the roll adjusting radius of another forming process is equal to the target transverse curvature radius of the forming part. Finite element analysis models are established; spherical and saddle surfaces are simulated. The corresponding experimental results are obtained. The dimensional accuracy of the forming parts using the two types of forming processes is compared, and the difference between the two types of forming processes for forming parts is analyzed through simulated results. The bendable roll rotates around its bent axis easily if its bending deformation is small; therefore, the forming process that the roll adjusting radius is much larger than the target transverse curvature radius of the surface part has relatively extensive application prospect. The comparison and analysis of the forming results may provide useful guidance on optimizing the three-dimensional rolling process for three-dimensional surface parts.