This article considers the application of video-based research to address methodological challenges for organizational scholars concerned with the sociomaterial foundations to work practice. In particular the claim that "all practices are always sociomaterial" raises a "problem of relevance"—that is, on what grounds can we select material to include in the analytic account when there is a vast array of material in each setting? Furthermore, how can we grasp the sociality of material objects that are often taken for granted and that drift in and out of view? We address these methodological questions drawing on ethnomethodology and conversation analysis, and by making use of video recordings of everyday work and organizing. We demonstrate the approach with data from two service settings and explore the analysis both of single cases and collections. To conclude, the article considers the distinctive contributions that these video-based studies have for our understanding of sociomateriality and organizational practice more generally.