This article advances the concept of spiritual citizenship to examine how some religiously active migrants employ religion to see themselves as, and to try to become, less deportable. Drawing from ethnographic observations and interviews with Central American and Mexican immigrants in the United States, I find that undocumented migrants use religion to redefine their own sense of self and to position themselves as spiritual citizens of “good moral character.” This research examines how the priorities of religious organizations can operate in relation to and through a neoliberal context. While religion supports migrants as they endure criminalization, my discussion of spiritual citizenship shows how the benefits of religious participation can also depend on migrants’ willingness to become deserving neoliberal citizens.